用溶胶一凝胶方法制备了纳米多晶La0.7Sr0.3MnO3样品.测量了不同温度下烧结的样品的零场冷却交流磁化率与温度和直流磁场的依赖关系.通过对铁磁-顺磁转变点附近临界峰的分析,得到973K烧结的多晶样品居里温度为312.1K±0.2K,临界指数为:δ=3.040,γ=1.007,β=0.493;1173K烧结的多晶样品居里温度为331.7K±0.1K,临界指数分别为:δ=2.950,γ=0.993,β=0.508.两组数据均与平均场理论预言结果一致,表明纳米多晶La0.7Sr0.3MnO3样品在磁性相变点附近存在长程相互作用.
参考文献
[1] | HELMOLT R VON;WECKER J;HOLZAPFEL B et al.Giant negative magnetoresistance in perovskitelike La2/3 Ba1/3 MnOx ferromagnetic films[J].Physical Review Letters,1993,71:2331-2333. |
[2] | JIN S;TIEFEL T H;MCCORMACK M et al.Thousandfold change in resistivity in magnetoresiative La-Ca-Mn-O Films[J].Science,1994,264:413-415. |
[3] | URUSHIBARA A;MORITOMO Y;ARIMA T et al.Insulator-met al transition and giant magnetoresistance in La1-x Srx MnO3[J].Physical Review B,1995,51:14103-14109. |
[4] | RAMIREZ A P .Colossal magnetoresistanee[J].Journal of Physics:Condensed Matter,1997,9:8171-8199. |
[5] | ZENER C .Interaction between the d-shells in the transition met als.Ⅱ Ferromagnetic compounds of manganese with perovskite structure[J].Physical Review,1951,82:403-405. |
[6] | MILLIS A J;LITTLEWOOD P B;SHRAlMAN B I .Double exchange alone does not explain the resistivity of La1-xSrx MnO3[J].Physical Review Letters,1995,74:5144-5147. |
[7] | Millis AJ. .COOPERATIVE JAHN-TELLER EFFECT AND ELECTRON-PHONON COUPLING IN LA(1-X)A(X)MNO(3)[J].Physical Review.B.Condensed Matter,1996(13):8434-8441. |
[8] | MORRISH A H.International conference on ferrites[M].Baltimore:University Park Press,1970 |
[9] | Lofland SE.;Kim PH.;Bhagat SM.;Manheimer MA.;Tyagi SD.;Ray V. .MAGNETIC PHASE TRANSITION IN LA0.7SR0.3MNO3 - MICROWAVE ABSORPTION STUDIES[J].Physical Review.B.Condensed Matter,1997(5):2749-2751. |
[10] | Ch.V. Mohan;M. Seeger;H. Kronmueller .Critical behaviour near the ferromagnetic-paramagnetic phase transition in La_(0.8)Sr_(0.2)MnO_(3)[J].Journal of Magnetism and Magnetic Materials,1998(3):348-355. |
[11] | Ghosh K.;Greene RL.;Karabashev SG.;Shulyatev DA.;Arsenov AA. Mukovskii Y.;Lobb CJ. .Critical phenomena in the double-exchange ferromagnet La0.7Sr0.3MnO3[J].Physical review letters,1998(21):4740-4743. |
[12] | WILUAMs G .Critical behaviour of some perovskites and pyrochlores:what's unusual and what's not[J].Journal of Alloys and Compounds,2001,326:36-46. |
[13] | Li W;Kunkel HP;Zhou XZ;Williams G;Mukovskii Y;Shulyatev D .Critical behavior of the field-dependent susceptibility in single-crystal La0.73Ba0.27MnO3[J].Physical review, B. Condensed matter and materials physics,2007(1):2406-1-2406-3-0. |
[14] | CHIKAZUMI S.Physics of Ferromagnetism[M].Oxford:clarendon Press,1997 |
[15] | STANLEY H E.Introduction to Phase Transitions and Critical Phenomena[M].Oxford:clarendon Press,1971 |
上一张
下一张
上一张
下一张
计量
- 下载量()
- 访问量()
文章评分
- 您的评分:
-
10%
-
20%
-
30%
-
40%
-
50%