欢迎登录材料期刊网

材料期刊网

高级检索

采集了太原市2013年4-12月大气干沉降样品,并使用了离子色谱仪分析了其中的水溶性无机阴阳离子,报道了干沉降中水溶性离子的化学特征、沉降通量和来源分析.结果表明,SO42-、Ca2+和NO3-是太原市干沉降的主要离子,浓度分别为4258.83、2388.45、1048.35 μg·g-1.干沉降中的水溶性离子浓度水平季节变化趋势为秋季>夏季>春季,变化趋势受到排放源和气象因素的影响.降尘通量和水溶性离子沉降通量分别为323.72 mg·(m2· d)-1和21.43 mg· (m2·d)-1.干沉降中硫、氮沉降通量分别为1.55 t·(km2·a)-1和0.39 t·(km2·a)-1,高于国内其他地区的研究结果.水溶性离子的相关性分析和特征比值结果显示,干沉降中的NO3-和SO42-主要受到燃煤排放影响;Ca2+和Mg2+的主要来源除了扬尘外,燃煤也有贡献.

参考文献

[1] Ying I. Tsai;Su-Ching Kuo;Li-Hao Young;Li-Ying Hsieh;Pei-Ti Chen.Atmospheric dry plus wet deposition and wet-only deposition of dicarboxylic acids and inorganic compounds in a coastal suburban environment[J].Atmospheric environment,2014Jun.(Jun.):696-706.
[2] 蔡阳阳;杨复沫;贺克斌;马永亮;奥田知明;田中茂.北京城区大气干沉降的水溶性离子特征[J].中国环境科学,2011(7):1071-1076.
[3] Li Li;Wu Wang;Jialiang Feng;Dongping Zhang;Huaijian Li;Zeping Gu;Bangjin Wang;Guoying Sheng;Jiamo Fu.Composition, source, mass closure of PM_(2.5) aerosols for four forests in eastern China[J].环境科学学报(英文版),2010(03):405-412.
[4] Fang GC;Wu YS;Chang SY;Rau JY;Huang SH.Dry deposition, ionic species measured and source interpretation during seasonal cycle at offshore areas near Taiwan Strait[J].Chemosphere: Environmental toxicology and risk assessment,20068(8):1253-1263.
[5] 潘月鹏;王跃思;杨勇杰;吴丹;辛金元;樊文雁.区域大气颗粒物干沉降采集及金属元素分析方法[J].环境科学,2010(3):553-559.
[6] 张仁健;浦一芬;徐永福;盛立芳;金井豊;太田充恒.青岛大气气溶胶的浓度分布和干沉降的观测研究[J].气候与环境研究,2004(2):390-395.
[7] 黄强;宋建中;彭平安.珠江三角洲大气干沉降金属元素浓度和来源分析[J].地球与环境,2013(5):498-505.
[8] Liu XueJun;Ju XiaoTang;Zhang Ying;He ChuNe;Kopsch J;Zhang FuSuo.Nitrogen deposition in agroecosystems in the Beijing area.[J].Agriculture, Ecosystems & Environment: An International Journal for Scientific Research on the Relationship of Agriculture and Food Production to the Biosphere,20061/4(1/4):370-377.
[9] 郭利利;崔阳;张桂香;闫雨龙;何秋生;王新明.太原市采暖期大气PM2.5中多环芳烃的污染特征[J].地球与环境,2015(2):198-204.
[10] 郭晓方;崔阳;王开扬;何秋生;王新明.近3年太原市夏季降水的化学特征研究[J].环境科学,2015(2):388-395.
[11] 贾小花;解静芳;马翔;邸志东;毋燕妮.太原市冬季PM2.5水溶性组分污染特征分析[J].中国环境科学,2013(4):599-604.
[12] Balestrini R.;Tartari G.;Galli L..Wet and dry atmospheric deposition at prealpine and alpine sites in northern Italy[J].Atmospheric environment,20009(9):1455-1470.
[13] Shilei Long;Jianrong Zeng;Yan Li;Liangman Bao;Lingling Cao;Ke Liu;Liang Xu.Characteristics of secondary inorganic aerosol and sulfate species in size-fractionated aerosol particles in Shanghai[J].环境科学学报(英文版),2014(05):1040-1051.
[14] Shucai Zhang;Wei Zhang;Yating Shen;Kaiyan Wang;Lianwu Hu;Xuejun Wang.Dry deposition of atmospheric polycyclic aromatic hydrocarbons (PAHs) in the southeast suburb of Beijing, China[J].Atmospheric research,20081/2(1/2):138-148.
[15] 姚孟伟;郭晓方;闫雨龙;张啸;何秋生;王新明.太原市降水化学特征及来源分析[J].环境工程学报,2014(11):4864-4870.
[16] De-Yin Huang;Yi-Gang Xu;Ben Zhou;Hui-Huang Zhang;Jiang-Bo Lan.Wet deposition of nitrogen and sulfur in Guangzhou, a subtropical area in South China[J].Environmental Monitoring and Assessment: An International Journal,20101/4(1/4):429-439.
[17] 商少凌.厦门海域大气气溶胶中磷的沉降通量[J].厦门大学学报,1997(01):106.
[18] Wang Y;Zhuang GS;Zhang XY;Huang K;Xu C;Tang AH;Chen JM;An ZS.The ion chemistry, seasonal cycle, and sources of PM2.5 and TSP aerosol in Shanghai[J].Atmospheric environment,200616(16):2935-2952.
[19] Chemical characterization of water-soluble aerosols in different residential environments of semi arid region of India[J].Journal of atmospheric chemistry,20092(2):121.
[20] Zhang XY.;Cao JJ.;Li LM.;Arimoto R.;Cheng Y.;Huebert B.;Wang D..Characterization of Atmospheric Aerosol over XiAn in the South Margin of the Loess Plateau, China[J].Atmospheric environment,200226(26):4189-4199.
[21] Shu-hui Cheng;Ling-xiao Yang;Xue-hua Zhou;Li-kun Xue;Xiao-mei Gao;Yang Zhou;Wen-xing Wang.Size-fractionated water-soluble ions, situ pH and water content in aerosol on hazy days and the influences on visibility impairment in Jinan, China[J].Atmospheric environment,201127(27):4631-4640.
[22] K. Osada;M. Kido;C. Nishita;K. Matsunaga;Y. Iwasaka;M. Nagatani;H. Nakada.Changes in ionic constituents of free tropospheric aerosol particles obtained at Mt. Norikura (2770 m a.s.l.), central Japan, during the Shurin period in 2000[J].Atmospheric environment,200235(35):5469-5477.
上一张 下一张
上一张 下一张
计量
  • 下载量()
  • 访问量()
文章评分
  • 您的评分:
  • 1
    0%
  • 2
    0%
  • 3
    0%
  • 4
    0%
  • 5
    0%