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通过在硝酸溶液中373 K回流AgMnO4和Mn(NO3)2的混合物制备了Ag-hollandite纳米线材料,并将其用于乙醇选择性氧化反应.X射线衍射谱表明所得材料的主要晶相为Ag-hollandite,但有少量的软锰矿形成.氮气吸附-脱附实验证实材料存在微孔结构.场发射扫描电镜和透射电镜观察表明纳米线长度为0.5~4.0 μm,直径为10~20 nm.Ag-hollandite纳米线是一种很有前途的乙醇选择性氧化制乙醛催化剂,503 K时在120 h的反应时间内,乙醇转化率为82%,乙醛选择性为95%.

参考文献

[1] De Guzman R N;Shen Y F;Shaw B R;Suib S L O' Young C L .[J].Chemistry of Materials,1993,5(10):1395.
[2] Chang F M;Jansen M .[J].Angewandte Chemie International Edition,1984,23(11):906.
[3] 胡蓉蓉,程易,XIE Lanying,谢兰英,王德峥.掺Ag对氧化锰八面体分子筛催化CO氧化性能的影响[J].催化学报,2007(05):463-468.
[4] Gac W .[J].Applied Catalysis B:Environmental,2007,75(1-2):107.
[5] Xia G G;Yin Y G;Willis W S;Wang J Y,Suib S L .[J].Journal of Catalysis,199?,185(01):91.
[6] Li, LY;King, DL .Synthesis and characterization of silver hollandite and its application in emission control[J].Chemistry of Materials,2005(17):4335-4343.
[7] Chen JL;Tang XF;Liu JL;Zhan ES;Li J;Huang XM;Shen WJ .Synthesis and characterization of Ag-hollandite nanofibers and its catalytic application in ethanol oxidation[J].Chemistry of Materials: A Publication of the American Chemistry Society,2007(17):4292-4299.
[8] Liu J;Makwana V;Cai J;Suib S L Aindow M .[J].Journal of Physical Chemistry B,2003,107(35):9185.
[9] Wang Z M;Tezuka S;Kanoh H .[J].CHEMISTRY OF MATERIALS,2001,13(02):530.
[10] Zhou H;Wang J Y;Chen X;O'Young C L Suib S L .[J].Microporous and Mesoporous Materials,1998,21(4-6):315.
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