The magnetic properties and the phase Transformation of Tb1-xPrxFe1.96 (x=0 to 0.7) compounds were studied by means of vibrating sample magnetometer(VSM), X-ray diffraction(XRD) and SEM back-scattered electron (BSE).The result indicates that the saturation magnetization σs of compounds along an easy axis decreases with the addition of Pr contents, which reduces from 77.24 Am2·kg-1 (x=0) to 11.84 Am2·kg-1 (x=0.5) and then returns to 37.14 Am2·kg-1 (x=0.7).The non-cubic phases appear when x exceeds 0.2, and the matrix of Tb1-xPrxFe1.96 compounds changes from (Tb, Pr)Fe2 phase with x=0 to (Tb, Pr)Fe3 phase with x=0.4, and at last to (Tb, Pr)2Fe17 phase in Tb0.3Pr0.7Fe1.96.Moreover, the structure of the compounds may become more complex with the increase of Pr content.
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