用Ti3SiC2粉末作为焊料,采用热压反应烧结连接法连接SiC,通过正交实验,研究了连接温度、高温保温时间、连接压力和连接层厚度对试样连接强度的影响,优选出的最佳工艺参数分别为:1 500℃,30 min,30MPa,150 μm.所得到的接头最大剪切强度为39.49 MPa.微观结构研究和成分分析表明:在界面处,发生了元素的扩散,促进了界面结合,有明显的反应扩散层.物相分析显示在高温、高压、氩气气氛以及使用石墨模具的条件下,Ti3SiC2与母材发生界面反应,实现界面结合.
参考文献
| [1] | 李荣久.陶瓷-金属复合材料[M].北京:冶金工业出版社,1995 |
| [2] | 张建军,李树杰.非氧化物陶瓷连接技术的进展[J].硅酸盐学报,2002(01):102-107. |
| [3] | 张利,李树杰,张建军,冀小强,张艳.SiC陶瓷连接工艺及焊料反应产物研究[J].稀有金属材料与工程,2003(03):224-227. |
| [4] | 张建军,李树杰,张艳.用Ti/Ag粉坯连接的SiC陶瓷界面[J].中国有色金属学报,2004(03):455-459. |
| [5] | 刘洪丽,李树杰.用有机聚合物连接碳化硅陶瓷及陶瓷基复合材料[J].硅酸盐学报,2004(10):1246-1251. |
| [6] | Jeitschko W;Nowotny H .The crystal structure of Ti3 SiC2-a new complex carbide[J].Monatshefte Fur Chemie,1967,98:329-337. |
| [7] | TANG Ke;WANG Chang-an;HUANG Yong et al.A study on reaction mechanism and growth of Ti3 SiC2synthesized by hot-pressing[J].Materials Science and Engineering A,2002,328:206-212. |
| [8] | Li J T;Miyamoto Y.Investigation on novel features during reactive synthesis of Ti3SiC2 ceramic[A].北京:清华大学出版社,1998:594-597. |
| [9] | Barsoum MW.;Elraghy T. .SYNTHESIS AND CHARACTERIZATION OF A REMARKABLE CERAMIC - TI3SIC2[J].Journal of the American Ceramic Society,1996(7):1953-1956. |
| [10] | Sun Z M;Zhou Y C .Synthesis of Ti3SiC2 powders by a solid-liquid method[J].Scripta Materialia,1999,41(01):61-66. |
| [11] | Gao N F;Miyamoto Y;Zhang D .Dense Ti3SiC2:prepared by reactive HIP[J].材料科学技术学报（英文版）,1999,34(10):4385-4391. |
| [12] | Pampuch R;Lis J;Stobierski L et al.Solid combustion synthesis of Ti3SiC2[J].Journal of the European Ceramic Society,1989,5(05):283-288. |
| [13] | El-Raghy T;Barsoum M W .Processing and mechanical properties of Ti3 SiC2 ( Ⅰ ):reaction path and microstructure evolution[J].Journal of the American Ceramic Society,1999,82(10):2849-2854. |
| [14] | 单辉祖.材料力学教材[M].北京:国防工业出版社,1989:134. |
| [15] | 陈艳林,梅炳初,朱教群.可加工陶瓷Ti3SiC2的合成和性能[J].硅酸盐通报,2003(03):74-77,96. |
| [16] | El-Raghy T.;Barsoum MW. .Diffusion kinetics of the carburization and silicidation of Ti3SiC2[J].Journal of Applied Physics,1998(1):112-119. |
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